Data-driven quantification and parameterization of cloud physics in general, and of aerosol-cloud interactions in particular, rely on input data from observations or detailed simulations. These data sources have complementary limitations in terms of their spatial and temporal coverage and resolution; simulation data has the advantage of readily providing causality but cannot represent the full process complexity. In order to base data-driven approaches on comprehensive information, we therefore need ways to integrate different data sources.  We discuss how the classical statistical technique of Gaussian-process emulation can be combined with specifically initialized ensembles of detailed cloud simulations (large-eddy simulations, LES) to provide a framework for evaluating data-driven descriptions of cloud characteristics and processes across different data sources. We specifically illustrate this approach for integrating LES and satellite data of aerosol-cloud interactions in subtropical stratocumulus cloud decks. We furthermore explore the extension of our framework to ground-based observations of Arctic mixed-phase clouds.@en

The effect of anthropogenic aerosol on the reflectivity of stratocumulus cloud decks through changes in cloud amount is a major uncertainty in climate projections. In frequently occurring nonprecipitating stratocumulus, cloud amount can decrease through aerosol-enhanced cloud-top mixing. The climatological relevance of this effect is debated because ship exhaust only marginally reduces stratocumulus amount. By comparing detailed numerical simulations with satellite analyses, we show that ship-track studies cannot be generalized to estimate the climatological forcing of anthropogenic aerosol. The ship track-derived sensitivity of the radiative effect of nonprecipitating stratocumulus to aerosol overestimates their cooling effect by up to 200%. The offsetting warming effect of decreasing stratocumulus amount needs to be taken into account if we are to constrain the cloud-mediated radiative forcing of anthropogenic aerosol.

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